Structural properties of human glycodelin A in water and in water-alcohol mixtures: a comparison with bovine beta-lactoglobulin A

Biochim Biophys Acta. 1999 May 18;1431(2):451-61. doi: 10.1016/s0167-4838(99)00074-6.

Abstract

Human glycodelin A (GdA) is a glycoprotein that is highly homologous to bovine beta-lactoglobulin A (beta-LgA) because the amino acid sequences are 50-60% identical. The structural characteristics of human GdA and beta-LgA were compared in water and 2-propanol/water solutions. Circular dichroism spectra reveal that in water the two proteins have a very similar beta-sheet secondary structure. In the presence of 2-propanol/water mixtures (up to 50% v/v) the alpha-helix structure of both proteins increases. A further increase in the alcohol percentage of the solvent (up to 80% v/v 2-propanol) causes the formation of a new folded tertiary structure containing mainly beta-sheet features. Synchrotron radiation small angle X-ray scattering indicates that, in a neutral pH aqueous solution, GdA is a dimer. Its radius of gyration value (Rg), 25.1+/-0.4 A, is greater than that of beta-LgA (21.1+/-0.3 A), probably because of the contribution of polysaccharides bound to Asn-28 and Asn-63 residues of GdA. Conversely, small angle X-ray scattering and gel permeation chromatography data on GdA in 2-propanol have revealed a massive aggregation of the protein.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • 2-Propanol
  • Animals
  • Cattle
  • Circular Dichroism
  • Glycodelin
  • Glycoproteins / chemistry*
  • Humans
  • Lactoglobulins / chemistry*
  • Pregnancy Proteins / chemistry*
  • Protein Conformation
  • Solubility
  • Solvents
  • Thermodynamics
  • Water
  • X-Ray Diffraction

Substances

  • Glycodelin
  • Glycoproteins
  • Lactoglobulins
  • PAEP protein, human
  • Pregnancy Proteins
  • Solvents
  • Water
  • 2-Propanol