Cloning of a gene encoding hydroxyquinol 1,2-dioxygenase that catalyzes both intradiol and extradiol ring cleavage of catechol

Biosci Biotechnol Biochem. 1999 May;63(5):859-65. doi: 10.1271/bbb.63.859.

Abstract

Two Escherichia coli transformants with catechol 1,2-dioxygenase activity were selected from a gene library of the benzamide-assimilating bacterium Arthrobacter species strain BA-5-17, which produces four catechol 1,2-dioxygenase isozymes. A DNA fragment isolated from one transformant contained a complete open reading frame (ORF). The deduced amino acid sequence of the ORF shared high identity with hydroxyquinol 1,2-dioxygenase. An enzyme expressed by the ORF was purified to homogeneity and characterized. When hydroxyquinol was used as a substrate, the purified enzyme showed 6.8-fold activity of that for catechol. On the basis of the sequence identity and substrate specificity of the enzyme, we concluded that the ORF encoded hydroxyquinol 1,2-dioxygenase. When catechol was used as a substrate, cis,cis-muconic acid and 2-hydroxymuconic 6-semialdehyde, which were products by the intradiol and extradiol ring cleavage activities, respectively, were produced. These results showed that the hydroxyquinol 1,2-dioxygenase reported here was a novel dioxygenase that catalyzed both the intradiol and extradiol cleavage of catechol.

MeSH terms

  • Amino Acid Sequence
  • Base Sequence
  • Catalysis
  • Catechols / metabolism*
  • Cloning, Molecular
  • Dioxygenases*
  • Hydrolysis
  • Molecular Sequence Data
  • Open Reading Frames
  • Oxygenases / genetics*
  • Oxygenases / isolation & purification
  • Oxygenases / metabolism
  • Phylogeny
  • Sequence Homology, Amino Acid
  • Substrate Specificity

Substances

  • Catechols
  • Oxygenases
  • Dioxygenases
  • hydroxyquinol 1,2-dioxygenase
  • catechol

Associated data

  • GENBANK/AB016258