Preparation, characterization and properties of sterically stabilized paclitaxel-containing liposomes

J Control Release. 2000 Jan 3;63(1-2):19-30. doi: 10.1016/s0168-3659(99)00166-2.

Abstract

Paclitaxel (Taxol) is a diterpenoid isolated from Taxus brevifolia, approved by the FDA for the treatment of ovarian and breast cancers. Due to its low solubility in water, it is clinically administered dissolved in Cremophor EL, (polyethoxylated castor oil) and ethanol, which cause serious side effects. Inclusion of paclitaxel in liposomal formulations has proved to be a good approach to eliminating this vehicle and improving the drug's antitumor efficacy. We prepared different conventional and PEGylated liposomes containing paclitaxel and determined encapsulation efficiency, physical stability and drug leakage in human plasma. The best conventional liposome formulation was composed of ePC/PG 9:1, while for PEGylated liposomes the best composition was ePC/PG/CHOL/PEG(5000)-DPPE 9:1:2:0.7. PEGylated liposomes were found to be less stable during storage than the corresponding conventional liposomes and to have lower drug release in human plasma at 37 degrees C. In vitro cytotoxic activities were evaluated on HT-29 human colon adenocarcinoma and MeWo melanoma cell lines. After 2 and 48 h, conventional liposomes had the same cytotoxicity as free paclitaxel, while PEGylated liposomes were as active as free drug, only after 48 h. Pharmacokinetics and biodistribution were evaluated in Balb/c mice after i.v. injection of paclitaxel, formulated in Cremophor EL or in conventional or in PEGylated liposomes. Encapsulation of paclitaxel in conventional liposomes produced marked differences over the free drug pharmacokinetics. PEGylated liposomes were long-circulating liposomes, with an increased t(1/2) beta 48.6 h, against t(1/2) beta 9.27 h of conventional liposomes. Biodistribution studies showed a considerable decrease in drug uptake in MPS-containing organs (liver and spleen) at 0.5 and 3 h after injection with PEGylated compared to conventional liposomes.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antineoplastic Agents, Phytogenic / administration & dosage*
  • Antineoplastic Agents, Phytogenic / chemistry
  • Antineoplastic Agents, Phytogenic / pharmacokinetics*
  • Antineoplastic Agents, Phytogenic / toxicity
  • Cholesterol / administration & dosage
  • Cholesterol / chemistry
  • Drug Carriers
  • Female
  • HT29 Cells / drug effects
  • Humans
  • Liposomes / toxicity
  • Macrophages / metabolism
  • Mice
  • Mice, Inbred BALB C
  • Paclitaxel / administration & dosage*
  • Paclitaxel / chemistry
  • Paclitaxel / pharmacokinetics*
  • Paclitaxel / toxicity
  • Phosphatidylcholines / administration & dosage
  • Phosphatidylcholines / chemistry
  • Phosphatidylethanolamines / administration & dosage
  • Phosphatidylethanolamines / chemistry
  • Polyethylene Glycols / administration & dosage
  • Polyethylene Glycols / chemistry
  • Succinimides / administration & dosage
  • Succinimides / chemistry
  • Tissue Distribution
  • Tumor Cells, Cultured

Substances

  • Antineoplastic Agents, Phytogenic
  • Drug Carriers
  • Liposomes
  • Phosphatidylcholines
  • Phosphatidylethanolamines
  • Succinimides
  • 1,2-dipalmitoyl-3-phosphatidylethanolamine
  • Polyethylene Glycols
  • polyethylene glycol bis(succinimidyl succinate)
  • Cholesterol
  • Paclitaxel