A novel carbohydrate:acceptor oxidoreductase from Microdochium nivale

Eur J Biochem. 2001 Feb;268(4):1136-42. doi: 10.1046/j.1432-1327.2001.01982.x.

Abstract

A Microdochium nivale carbohydrate:acceptor oxidoreductase was purified, cloned, heterologously expressed, and characterized. The gene encoding the protein showed one intron, and the ORF showed a sequence with low homology (< or = 25% identity or 65% similarity) to other known flavin-containing carbohydrate oxidases. The maturation of the protein required the cleavage of a tetrameric propeptide in addition to an 18 amino-acid signal peptide. The enzyme was found to have a relative molecular mass of 55 000 Da, an isoelectric point of 9, and one FAD per protein. It could oxidize mono-, oligo-, or polymeric saccharides, and transfer their electrons to O2 or other acceptors. When D-glucose served as electron-donating substrate, an activity of 2 s(-1) was observed at pH 5.5 and 23 degrees C. Among various oligosaccharides, the enzyme preferred tetrameric dextrins, indicating a favorable interaction of four linked glucose units with the substrate pocket. The unique structure and ability of oxidizing oligo/polymeric saccharides suggest a promising prospect of this enzyme for various industrial/medicinal applications.

MeSH terms

  • Alcohol Oxidoreductases / chemistry
  • Alcohol Oxidoreductases / genetics*
  • Alcohol Oxidoreductases / metabolism
  • Amino Acid Sequence
  • Base Sequence
  • Carbohydrate Dehydrogenases / chemistry
  • Carbohydrate Dehydrogenases / genetics*
  • Carbohydrate Dehydrogenases / metabolism
  • Carbohydrate Metabolism
  • Cloning, Molecular
  • Dextrins / metabolism
  • Fungal Proteins*
  • Isoelectric Point
  • Molecular Sequence Data
  • Molecular Weight
  • Sordariales / enzymology*
  • Sordariales / genetics

Substances

  • Dextrins
  • Fungal Proteins
  • Alcohol Oxidoreductases
  • Carbohydrate Dehydrogenases
  • MnCO protein, Microdochium nivale