Kinetics study of the biotransformation of an oligonucleotide prodrug in cells extract by matrix-assisted laser desorption-ionization time-of-flight mass spectrometry

J Chromatogr B Biomed Sci Appl. 2001 Mar 25;753(1):123-30. doi: 10.1016/s0378-4347(00)00502-8.

Abstract

The fate of a dodecathymidine prodrug in cell extract was monitored by MALDI-TOF MS. This technique allows a facile identification and a relative quantification of metabolites produced. We showed that the relative peak intensities were similar to the relative metabolite proportions that permitted the determination of their half-lives. We found a good fit between the calculated kinetics curves and the experimental points. The oligonucleotide prodrug was fully metabolized to yield the dodecathymidine phosphorothioate likely through a carboxyesterase mediated mechanism.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biotransformation
  • Cell Extracts*
  • Oligonucleotides / chemistry
  • Oligonucleotides / pharmacokinetics*
  • Prodrugs / pharmacokinetics*
  • Spectrometry, Mass, Matrix-Assisted Laser Desorption-Ionization
  • Thymidine / chemistry

Substances

  • Cell Extracts
  • Oligonucleotides
  • Prodrugs
  • Thymidine