Reversal of cisplatin and multidrug resistance by ribozyme-mediated glutathione suppression

Biochem Biophys Res Commun. 2001 Aug 17;286(2):406-13. doi: 10.1006/bbrc.2001.5399.

Abstract

gamma-Glutamylcysteine synthetase (gamma-GCS) is a key enzyme in glutathione (GSH) synthesis, and is thought to play a significant role in intracellular detoxification, especially of anticancer drugs. Increased levels of GSH are commonly found in the drug-resistant human cancer cells. We designed a hammerhead ribozyme against gamma-GCS mRNA (anti-gamma-GCS Rz), which specifically down-regulated gamma-GCS gene expression in the HCT-8 human colon cancer cell line. The aim of this study was to reverse the cisplatin and multidrug resistance for anticancer drugs. The cisplatin-resistant HCT-8 cells (HCT-8DDP cells) overexpressed MRP and MDR1 genes, and showed resistance to not only cisplatin (CDDP), but also doxorubicin (DOX) and etoposide (VP-16). We transfected a vector expressing anti-gamma-GCS Rz into the HCT-8DDP cells (HCT-8DDP/Rz). The anti-gamma-GCS Rz significantly suppressed MRP and MDR, and altered anticancer drug resistance. The HCT-8DDP/Rz cells were more sensitive to CDDP, DOX and VP-16 by 1.8-, 4.9-, and 1.5-fold, respectively, compared to HCT-8DDP cells. The anti-gamma-GCS Rz significantly down-regulated gamma-GCS gene expression as well as MRP/MDR1 expression, and reversed resistance to CDDP, DOX and VP-16. These results suggested that gamma-GCS plays an important role in both cisplatin and multidrug resistance in human cancer cells.

MeSH terms

  • Antineoplastic Agents / therapeutic use*
  • Cisplatin / therapeutic use*
  • Colonic Neoplasms / genetics
  • Colonic Neoplasms / metabolism
  • Colonic Neoplasms / therapy*
  • Drug Resistance, Multiple
  • Drug Resistance, Neoplasm
  • Glutamate-Cysteine Ligase / genetics
  • Glutathione / antagonists & inhibitors*
  • Humans
  • RNA, Catalytic / therapeutic use*
  • RNA, Neoplasm / biosynthesis
  • RNA, Neoplasm / genetics
  • Tetrazolium Salts / chemistry
  • Thiazoles / chemistry
  • Tumor Cells, Cultured

Substances

  • Antineoplastic Agents
  • RNA, Catalytic
  • RNA, Neoplasm
  • Tetrazolium Salts
  • Thiazoles
  • Glutamate-Cysteine Ligase
  • thiazolyl blue
  • Glutathione
  • Cisplatin