Characterization of a functional soluble form of a Brassica napus membrane-anchored endo-1,4-beta-glucanase heterologously expressed in Pichia pastoris

Plant Physiol. 2001 Oct;127(2):674-84. doi: 10.1104/pp.010269.

Abstract

The Brassica napus gene, Cel16, encodes a membrane-anchored endo-1,4-beta-glucanase with a deduced molecular mass of 69 kD. As for other membrane-anchored endo-1,4-beta-glucanases, Cel16 consists of a predicted intracellular, charged N terminus (methionine(1)-lysine(70)), a hydrophobic transmembrane domain (isoleucine(71)-valine(93)), and a periplasmic catalytic core (lysine(94)-proline(621)). Here, we report the functional analysis of Delta(1-90)Cel16, the N terminally truncated Cel16, missing residues 1 through 90 and comprising the catalytic domain of Cel16 expressed recombinantly in the methylotrophic yeast Pichia pastoris as a soluble protein. A two-step purification protocol yielded Delta(1-90)Cel16 in a pure form. The molecular mass of Delta(1-90)Cel16, when determined by sodium dodecyl sulfate-polyacrylamide gel electrophoresis, was about 130 kD and about 60 kD after enzymatic removal of N-glycans, fitting the expected molecular mass of 59 kD. Delta(1-90)Cel16 was highly N glycosylated as compared with the native B. napus Cel16 protein. Delta(1-90)Cel16 had a pH optimum of 6.0. The activity of Delta(1-90)Cel16 was inhibited by EDTA and exhibited a strong dependence on calcium. Delta(1-90)Cel16 showed substrate specificity for low substituted carboxymethyl-cellulose and amorphous cellulose. It did not hydrolyze crystalline cellulose, xyloglycan, xylan, (1-->3),(1-->4)-beta-D-glucan, the highly substituted hydroxyethylcellulose, or the oligosaccharides cellotriose, cellotetraose, cellopentaose, or xylopentaose. Size exclusion analysis of Delta(1-90)Cel16-hydrolyzed carboxymethylcellulose showed that Delta(1-90)Cel16 is a true endo-acting glucanase.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Antibodies, Heterophile
  • Brassica napus / enzymology*
  • Brassica napus / genetics
  • Brassica napus / growth & development
  • Calcium / pharmacology
  • Carboxymethylcellulose Sodium
  • Catalysis
  • Cell Membrane / enzymology
  • Cellulase / genetics
  • Cellulase / isolation & purification
  • Cellulase / metabolism*
  • Cellulose / metabolism*
  • Cloning, Molecular
  • Edetic Acid / pharmacology
  • Gene Expression Regulation, Enzymologic / physiology
  • Gene Expression Regulation, Plant / physiology
  • Hydrogen-Ion Concentration
  • Magnesium / pharmacology
  • Membrane Proteins / genetics
  • Membrane Proteins / isolation & purification
  • Membrane Proteins / metabolism*
  • Molecular Sequence Data
  • Pichia / genetics*
  • Plant Proteins / genetics
  • Solubility
  • Substrate Specificity
  • Zinc / pharmacology

Substances

  • Antibodies, Heterophile
  • Membrane Proteins
  • Plant Proteins
  • Cellulose
  • Edetic Acid
  • Cel16 protein, Brassica napus
  • Cellulase
  • Magnesium
  • Zinc
  • Carboxymethylcellulose Sodium
  • Calcium