Biomimetic synthesis of a water soluble conducting molecular complex of polyaniline and lignosulfonate

Biomacromolecules. 2002 Sep-Oct;3(5):937-41. doi: 10.1021/bm0255138.

Abstract

A new biomimetic route for the synthesis of a conducting molecular complex of polyaniline (Pani) and a natural polyelectrolyte, lignosulfonate (LGS) is presented. A poly(ethylene glycol) modified hematin (PEG-hematin) was used to catalyze the polymerization of aniline in the presence of LGS to form a Pani/LGS complex. UV-vis, FTIR, conductivity and TGA studies for the LGS-polyaniline complex indicate the presence of a thermally stable and electrically conductive form of polyaniline. Also the presence of LGS in this complex, an inexpensive byproduct from pulp processing, provides a unique combination of properties such as electronic conductivity, processability and biodegradability. The use of this conductive complex for corrosion protection is also proposed.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Aniline Compounds / chemical synthesis*
  • Aniline Compounds / chemistry
  • Biodegradation, Environmental
  • Corrosion
  • Electric Conductivity
  • Hemin / chemistry
  • Lignin / analogs & derivatives*
  • Lignin / chemical synthesis*
  • Lignin / chemistry
  • Polymers / chemistry
  • Solubility
  • Temperature

Substances

  • Aniline Compounds
  • Polymers
  • polyaniline
  • Hemin
  • lignosulfuric acid
  • Lignin