Evaluation of enzymatic digestion and liquid chromatography-mass spectrometry peptide mapping of the integral membrane protein bacteriorhodopsin

Electrophoresis. 2002 Sep;23(18):3224-32. doi: 10.1002/1522-2683(200209)23:18<3224::AID-ELPS3224>3.0.CO;2-#.

Abstract

A method for the complete peptide mapping of the model integral membrane protein bacteri-orhodopsin is demonstrated. Utilizing more effective enzymatic digestion, procedures with capillary liquid chromatography-electrospray ionization-mass spectrometry (LC-ESI-MS) and tandem mass spectrometry (MS/MS), all predicted tryptic digestion products were detected, as well as peptides from all previously reported post-translational modifications of bacteriorhodopsin. A significant contribution of chymotryptic-like digestion products was also observed. A characterization of the behavior of hydrophobic integral membrane peptides in a reversed-phase liquid chromatographic separation is also provided. The method reported here offers improved compatibility of the solubilizing reagents with both the chromatography and mass spectrometry, rendering it suitable for high-throughput proteomic applications.

Publication types

  • Evaluation Study
  • Research Support, U.S. Gov't, Non-P.H.S.
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amino Acid Sequence
  • Bacteriorhodopsins / chemistry*
  • Bacteriorhodopsins / genetics
  • Chromatography, Liquid / methods*
  • Mass Spectrometry / methods*
  • Models, Molecular
  • Molecular Sequence Data
  • Peptide Fragments / analysis
  • Peptide Fragments / genetics
  • Peptide Mapping / methods*
  • Protein Structure, Secondary
  • Spectrometry, Mass, Electrospray Ionization / methods
  • Trypsin

Substances

  • Peptide Fragments
  • Bacteriorhodopsins
  • Trypsin