The inhibition of phosphatidylinositol 3-kinase by quercetin and analogs

Biochem Biophys Res Commun. 1992 Jul 31;186(2):624-31. doi: 10.1016/0006-291x(92)90792-j.

Abstract

Phosphatidylinositol (PtdIns) 3-kinase is an enzyme involved in cellular responses to growth factors. Quercetin (2-(3,4-dihydroxyphenyl)-3,5,7-trihydroxy-4H-1-benzopyrano-4-one), a naturally occuring bioflavinoid, was found to inhibit PtdIns 3-kinase with an IC50 of 1.3 micrograms/ml (3.8 microM); inhibition appears to be directed towards the ATP binding site of the kinase. Analogs of quercetin were also investigated as PtdIns 3-kinase inhibitors, with the most potent compounds exhibiting IC50's in the range of 1.7-8.4 micrograms/ml (5-19 microM). In contrast, genistein, a potent tyrosine kinase inhibitor of the isoflavone class, did not inhibit PtdIns 3-kinase significantly (IC50 greater than 30 micrograms/ml). These findings suggest that flavinoids may serve as potent inhibitors of PtdIns 3-kinase. Furthermore, the enzyme is much more sensitive to substituents at the 3-position of the flavinoid ring than are other protein and PtdIns kinases, suggesting that specific inhibitors of PtdIns 3-kinase can be developed to explore the biological role of the enzyme in cellular proliferation and growth factor response.

Publication types

  • Comparative Study

MeSH terms

  • Animals
  • Brain / enzymology
  • Cattle
  • Flavonoids / pharmacology*
  • Kinetics
  • Molecular Structure
  • Phosphatidylinositol 3-Kinases
  • Phosphotransferases / antagonists & inhibitors*
  • Phosphotransferases / isolation & purification
  • Quercetin / analogs & derivatives*
  • Quercetin / pharmacology*
  • Structure-Activity Relationship

Substances

  • Flavonoids
  • Quercetin
  • Phosphotransferases
  • Phosphatidylinositol 3-Kinases