Sequential binding of agonists to the beta2 adrenoceptor. Kinetic evidence for intermediate conformational states

J Biol Chem. 2004 Jan 2;279(1):686-91. doi: 10.1074/jbc.M310888200. Epub 2003 Oct 14.

Abstract

The beta2 adrenoreceptor (beta2AR) is a prototypical G protein-coupled receptor (GPCR) activated by catecholamines. Agonist activation of GPCRs leads to sequential interactions with heterotrimeric G proteins, which activate cellular signaling cascades, and with GPCR kinases and arrestins, which attenuate GPCR-mediated signaling. We used fluorescence spectroscopy to monitor catecholamine-induced conformational changes in purified beta2AR. Here we show that upon catecholamine binding, beta2ARs undergo transitions to two kinetically distinguishable conformational states. Using a panel of chemically related catechol derivatives, we identified the specific chemical groups on the agonist responsible for the rapid and slow conformational changes in the receptor. The conformational changes observed in our biophysical assay were correlated with biologic responses in cellular assays. Dopamine, which induces only a rapid conformational change, is efficient at activating Gs but not receptor internalization. In contrast, norepinephrine and epinephrine, which induce both rapid and slow conformational changes, are efficient at activating Gs and receptor internalization. These results support a mechanistic model for GPCR activation where contacts between the receptor and structural determinants of the agonist stabilize a succession of conformational states with distinct cellular functions.

MeSH terms

  • Adrenergic beta-Agonists / metabolism*
  • Animals
  • Binding Sites
  • Catechols / metabolism
  • Dopamine / metabolism
  • Epinephrine / metabolism
  • Isoproterenol / metabolism
  • Kinetics
  • Models, Molecular
  • Norepinephrine / metabolism
  • Protein Conformation
  • Receptors, Adrenergic, beta-2 / chemistry*
  • Receptors, Adrenergic, beta-2 / physiology*
  • Spectrometry, Fluorescence
  • Spodoptera
  • Transfection

Substances

  • Adrenergic beta-Agonists
  • Catechols
  • Receptors, Adrenergic, beta-2
  • Isoproterenol
  • catechol
  • Dopamine
  • Norepinephrine
  • Epinephrine