The crystal structure of murine CMP-5-N-acetylneuraminic acid synthetase

J Mol Biol. 2003 Dec 5;334(4):625-37. doi: 10.1016/j.jmb.2003.09.080.

Abstract

Sialic acids are activated by CMP-5-N-acetylneuraminic acid synthetase prior to their transfer onto oligo- or polysaccharides. Here, we present the crystal structure of the N-terminal catalytically active domain of the murine 5-N-acetylneuraminic acid synthetase in complex with the reaction product. In contrast to the previously solved structure of 5-N-acetylneuraminic acid synthetase from Neisseria meningitidis and the related CMP-KDO-synthetase of Escherichia coli, the murine enzyme is a tetramer, which was observed with the active sites closed. In this conformation a loop is shifted by 6A towards the active site and thus an essential arginine residue can participate in catalysis. Furthermore, a network of intermolecular salt-bridges and hydrogen bonds in the dimer as well as hydrophobic interfaces between two dimers indicate a cooperative behaviour of the enzyme. In addition, a complex regulation of the enzyme activity is proposed that includes phosphorylation and dephosphorylation.

MeSH terms

  • Amino Acid Sequence
  • Animals
  • Bacterial Proteins / chemistry
  • Bacterial Proteins / metabolism
  • Binding Sites
  • Crystallography, X-Ray
  • Cytidine Monophosphate N-Acetylneuraminic Acid / chemistry
  • Cytidine Monophosphate N-Acetylneuraminic Acid / metabolism
  • Humans
  • Mice
  • Models, Molecular
  • Molecular Sequence Data
  • Molecular Structure
  • N-Acylneuraminate Cytidylyltransferase / chemistry*
  • N-Acylneuraminate Cytidylyltransferase / metabolism
  • Protein Binding
  • Protein Conformation
  • Protein Folding
  • Protein Structure, Quaternary*
  • Protein Structure, Secondary
  • Protein Structure, Tertiary
  • Sequence Alignment

Substances

  • Bacterial Proteins
  • Cytidine Monophosphate N-Acetylneuraminic Acid
  • N-Acylneuraminate Cytidylyltransferase

Associated data

  • PDB/1QWJ