A new cucurbitacin D related 16,23-epoxy derivative and its isomerization products

Org Lett. 2004 Feb 19;6(4):633-6. doi: 10.1021/ol036469r.

Abstract

[reaction: see text] A new (23S,24Z)-16,23-epoxy cucurbitacin derivative was isolated from Ecballium elaterium L. (Cucurbitaceae) fruit juice along with known cucurbitacin derivatives. Structure elucidation of these derivatives was accomplished by NMR spectroscopy and mass spectrometry from HPLC-MS data. Isomerization of the epoxy derivative was monitored by 1D and 2D NMR experiments. The configuration of the reaction products was elucidated as (23R,24E) and (23R,24Z), and a mechanism for the acid-catalyzed rearrangement process is proposed.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Chromatography, High Pressure Liquid
  • Cucurbitaceae / chemistry*
  • Epoxy Compounds / chemistry
  • Epoxy Compounds / isolation & purification
  • Fruit / chemistry
  • Molecular Structure
  • Nuclear Magnetic Resonance, Biomolecular
  • Plants, Medicinal / chemistry*
  • Stereoisomerism
  • Triterpenes / chemistry*
  • Triterpenes / isolation & purification*

Substances

  • Epoxy Compounds
  • Triterpenes
  • cucurbitacin D