Structural analysis of hydroperoxy- and epoxy-triacylglycerols by liquid chromatography mass spectrometry

Chem Phys Lipids. 2004 Aug;131(1):41-9. doi: 10.1016/j.chemphyslip.2004.03.008.

Abstract

Oxidation of triacylglycerols (TAGs) containing oleic acid leads to the formation of several products. This study characterizes hydroperoxy- and epoxy-TAGs including their regio-isomers. For this purpose, epoxy- and hydroperoxy-TAGs, formed by oxidation of 1,2-dipalmitoyl-3-oleoyl-glycerol (PPO) and 1,3-dipalmitoyl-2-oleoyl-glycerol (POP) under air and 18O2, were analysed by reverse phase liquid chromatography-electrospray ionisation-mass spectrometry (LC-ESI-MS) using a triple quadrupole mass analyser, in positive ion mode. Post-column infusion of ammonium formiate was used to obtain intense molecular ion adducts. Pure 1,2-dipalmitoyl-3-epoxystearoyl-glycerol (PPEs) and 1,3-dipalmitoyl-2-epoxystearoyl-glycerol (PEsP), synthesized by epoxidation of the corresponding monounsaturated TAGs, were used to confirm MS/MS identification. The use of 18O2 oxidation experiments permitted unambiguous identification of MS/MS fragmentation pathways of both hydroperoxide and epoxy-TAGs. Fragmentation of hydroperoxy-TAGs are very distinct from their epoxy-TAGs homologues and consist of simultaneous losses of hydrogen peroxide (34 a.m.u.) and water (18 a.m.u.).

MeSH terms

  • Air*
  • Chromatography, Liquid / methods
  • Epoxy Compounds / chemistry
  • Fatty Acids, Monounsaturated / chemistry
  • Isomerism
  • Mass Spectrometry / methods*
  • Oleic Acid / chemistry
  • Oxidation-Reduction
  • Stearic Acids / chemistry
  • Triglycerides / analysis
  • Triglycerides / chemistry*
  • Water / chemistry*

Substances

  • Epoxy Compounds
  • Fatty Acids, Monounsaturated
  • Stearic Acids
  • Triglycerides
  • Water
  • Oleic Acid
  • stearic acid