Novel biodegradable copolyesters containing blocks of poly(3-hydroxyoctanoate) and poly(epsilon-caprolactone): synthesis and characterization

Macromol Biosci. 2004 Nov 20;4(11):1014-20. doi: 10.1002/mabi.200400104.

Abstract

Novel biodegradable polyester block copolymers have been synthesized by using well-defined poly(3-hydroxyoctanoate) (PHO) oligomers having a hydroxyl end group and an ester end group with M(n) values of 800, 2,500, 5,300, 8,000, or 20,000 as an elastomeric soft segment and poly(epsilon-caprolactone) as a more crystalline segment. These PHO oligomers prepared by methanolysis were subjected to block copolymerization with epsilon-caprolactone. The chemical structure of the copolymers was confirmed by (1)H NMR and (13)C NMR spectroscopy. All the copolyesters are semi-crystalline and two T(g) were observed by differential scanning calorimetry when the molecular weight of the PHO block is about 20,000.

MeSH terms

  • Animals
  • Biocompatible Materials / chemical synthesis
  • Biocompatible Materials / chemistry
  • Biocompatible Materials / metabolism
  • Biodegradation, Environmental
  • Caprylates / chemistry*
  • Caprylates / metabolism
  • Drug Delivery Systems
  • Magnetic Resonance Spectroscopy
  • Molecular Structure
  • Polyesters / chemical synthesis
  • Polyesters / chemistry*
  • Polyesters / metabolism

Substances

  • Biocompatible Materials
  • Caprylates
  • Polyesters
  • polycaprolactone
  • 3-hydroxyoctanoic acid