Identification of pathway-selective estrogen receptor ligands that inhibit NF-kappaB transcriptional activity

Proc Natl Acad Sci U S A. 2005 Feb 15;102(7):2543-8. doi: 10.1073/pnas.0405841102. Epub 2005 Feb 7.

Abstract

Inflammation is now recognized as a key component in a number of diseases such as atherosclerosis, rheumatoid arthritis, and inflammatory bowel disease. The transcription factor NF-kappaB has been shown to be involved in both the early and late stages of the inflammatory-proliferative process. In this report, we describe the identification of the pathway-selective estrogen receptor (ER) ligand, WAY-169916, that inhibits NF-kappaB transcriptional activity but is devoid of conventional estrogenic activity. This pathway-selective ligand does not promote the classic actions of estrogens such as stimulation of uterine proliferation or ER-mediated gene expression, but is a potent antiinflammatory agent, as demonstrated in the HLA-B27 transgenic rat model of inflammatory bowel disease. Our results indicate the potential utility of pathway-selective ER ligands such as WAY-169916 in the treatment of chronic inflammatory diseases.

MeSH terms

  • Animals
  • Animals, Genetically Modified
  • Cell Line
  • Estrogen Receptor alpha / genetics
  • Estrogen Receptor alpha / metabolism
  • Estrogen Receptor beta / genetics
  • Estrogen Receptor beta / metabolism
  • Female
  • HLA-B27 Antigen / genetics
  • Humans
  • Inflammatory Bowel Diseases / drug therapy
  • Inflammatory Bowel Diseases / genetics
  • Inflammatory Bowel Diseases / metabolism
  • Ligands
  • Male
  • Mice
  • Mice, Inbred C57BL
  • NF-kappa B / antagonists & inhibitors*
  • Pyrazoles / chemistry
  • Pyrazoles / metabolism*
  • Pyrazoles / pharmacology*
  • Rats
  • Receptors, Estrogen / metabolism*
  • Transcription, Genetic / drug effects*
  • Uterus / drug effects
  • Uterus / metabolism

Substances

  • Estrogen Receptor alpha
  • Estrogen Receptor beta
  • HLA-B27 Antigen
  • Ligands
  • NF-kappa B
  • Pyrazoles
  • Receptors, Estrogen
  • WAY-169916