Lower induction of p53 and decreased apoptosis in NQO1-null mice lead to increased sensitivity to chemical-induced skin carcinogenesis

Cancer Res. 2005 Mar 15;65(6):2054-8. doi: 10.1158/0008-5472.CAN-04-3157.

Abstract

NAD(P)H:quinone oxidoreductase 1 (NQO1) is a cytosolic protein that catalyzes metabolic detoxification of quinones and protects cells against redox cycling and oxidative stress. NQO1-null mice deficient in NQO1 protein showed increased sensitivity to 7,12-dimethylbenz(a)anthracene- and benzo(a)pyrene-induced skin carcinogenesis. In the present studies, we show that benzo(a)pyrene metabolite benzo(a)pyrene-trans-7,8-dihydrodiol-9,10-epoxide and not benzo(a)pyrene quinones contributed to increased benzo(a) pyrene-induced skin tumors in NQO1-null mice. An analysis of untreated skin revealed an altered intracellular redox state due to accumulation of NADH and reduced levels of NAD/NADH in NQO1-null mice as compared with wild-type mice. Treatment with benzo(a)pyrene failed to significantly increase p53 and apoptosis in the skin of NQO1-null mice when compared with wild-type mice. These results led to the conclusion that altered intracellular redox state along with lack of induction of p53 and decreased apoptosis plays a significant role in increased sensitivity of NQO1-null mice to benzo(a)pyrene-induced skin cancer.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • 7,8-Dihydro-7,8-dihydroxybenzo(a)pyrene 9,10-oxide / pharmacokinetics
  • Animals
  • Apoptosis / drug effects
  • Apoptosis / physiology*
  • Benzo(a)pyrene / pharmacokinetics*
  • Carcinogens / pharmacokinetics
  • Female
  • Inactivation, Metabolic
  • Male
  • Mice
  • Mice, Inbred C57BL
  • NAD / metabolism
  • NAD(P)H Dehydrogenase (Quinone)
  • NADPH Dehydrogenase / deficiency*
  • NADPH Dehydrogenase / metabolism
  • Oxidation-Reduction
  • Skin / drug effects
  • Skin / enzymology
  • Skin / metabolism
  • Skin Neoplasms / chemically induced*
  • Skin Neoplasms / enzymology*
  • Skin Neoplasms / metabolism
  • Tetradecanoylphorbol Acetate
  • Tumor Suppressor Protein p53 / biosynthesis*

Substances

  • Carcinogens
  • Tumor Suppressor Protein p53
  • NAD
  • Benzo(a)pyrene
  • 7,8-Dihydro-7,8-dihydroxybenzo(a)pyrene 9,10-oxide
  • NAD(P)H Dehydrogenase (Quinone)
  • Nqo1 protein, mouse
  • NADPH Dehydrogenase
  • Tetradecanoylphorbol Acetate