Cell-dependent interference of a series of new 6-aminoquinolone derivatives with viral (HIV/CMV) transactivation

J Antimicrob Chemother. 2005 Nov;56(5):847-55. doi: 10.1093/jac/dki328. Epub 2005 Sep 8.

Abstract

Objectives: Quinolone derivatives have been shown to inhibit human immunodeficiency virus (HIV) replication at the transcriptional level. Recently, a series of new 6-aminoquinolones that are endowed with more pronounced anti-HIV activities compared with the formerly reported quinolone derivatives have been published. These potent 6-aminoquinolones were further evaluated for their broad-spectrum antiviral properties.

Methods: Latently HIV-1-infected cell lines as well as cytomegalovirus (CMV)-infected fibroblasts were used to evaluate the antiviral potency of the 6-aminoquinolone derivatives. Additionally green fluorescent protein (GFP) transactivation experiments using different promoters were conducted.

Results: The compounds completely suppressed tumour necrosis factor alpha (TNF-alpha)- and phorbol 12-myristate 13-acetate (PMA)-induced HIV-1 expression in latently HIV-1-infected OM-10.1 and U1 cell lines at non-toxic concentrations. In addition, HIV-1 mRNA production was dramatically suppressed in both cell lines in a dose-dependent manner. In the same concentration range, the compounds inhibited TNF-alpha release from PMA-induced OM-10.1 cells but allowed TNF-alpha production from PMA-induced U1 cells at all concentrations tested. The 6-aminoquinolone derivatives were not only inhibitory to the Tat-mediated transactivation of the HIV-1 LTR promoter, but were also found to interfere in a cell-dependent way with the transactivation process mediated from the human CMV immediate early and the human EF-1alpha promoter. Additionally, the 6-aminoquinolone derivatives were also found to be inhibitory to CMV replication in fibroblast cells.

Conclusions: It thus appears that the antiviral spectrum of this class of compounds is not confined to the specific inhibition of HIV but encompasses CMV as well. This broad-spectrum activity window might provide an interesting platform for future applications for the 6-aminoquinolone derivatives.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Aminoquinolines / chemistry
  • Aminoquinolines / pharmacology*
  • Animals
  • Antiviral Agents / pharmacology*
  • Cell Line
  • Cytomegalovirus / drug effects*
  • Cytomegalovirus / physiology
  • Genes, Immediate-Early
  • Green Fluorescent Proteins / analysis
  • HIV / drug effects*
  • HIV / genetics
  • HIV / physiology
  • HIV Long Terminal Repeat
  • Humans
  • Mice
  • Peptide Elongation Factor 1 / genetics
  • Promoter Regions, Genetic
  • RNA, Messenger / analysis
  • RNA, Viral / analysis
  • Tetradecanoylphorbol Acetate / analogs & derivatives
  • Tetradecanoylphorbol Acetate / pharmacology
  • Transcription, Genetic
  • Transcriptional Activation / drug effects*
  • Tumor Necrosis Factor-alpha / metabolism
  • Virus Activation
  • Virus Latency
  • Virus Replication / drug effects

Substances

  • Aminoquinolines
  • Antiviral Agents
  • Peptide Elongation Factor 1
  • RNA, Messenger
  • RNA, Viral
  • Tumor Necrosis Factor-alpha
  • Green Fluorescent Proteins
  • phorbolol myristate acetate
  • aminoquinolone
  • Tetradecanoylphorbol Acetate