Suppression of mast cell degranulation by a novel ceramide kinase inhibitor, the F-12509A olefin isomer K1

Biochim Biophys Acta. 2005 Dec 30;1738(1-3):82-90. doi: 10.1016/j.bbalip.2005.10.007. Epub 2005 Nov 14.

Abstract

Antigen-induced degranulation of mast cells plays a pivotal role in allergic and inflammatory responses. Recently, ceramide kinase (CERK) and its phosphorylated product ceramide 1-phosphate (C1P) have emerged as important players in mast cell degranulation. Here, we describe the synthesis of a novel F-12509A olefin isomer, K1, as an effective CERK inhibitor. In vitro kinase assays demonstrated that K1 effectively inhibits CERK without inhibiting sphingosine kinase and diacylglycerol kinase. Treating RBL-2H3 cells with K1 reduced cellular C1P levels to 40% yet had no effect on cell growth. Furthermore, treatment with K1 significantly suppressed both calcium ionophore- and IgE/antigen-induced degranulation, indicating that K1 interferes with signals that happen downstream of Ca(2+) mobilization. Finally, we show that K1 affects neither IgE/antigen-induced global tyrosine phosphorylation nor subsequent Ca(2+) elevation, suggesting a specificity for CERK-mediated signals. Our novel CERK inhibitor provides a useful tool for studying the biological functions of CERK and C1P. Moreover, to our knowledge, this is the first report demonstrating that inhibition of CERK suppresses IgE/antigen-induced mast cell degranulation. This finding suggests that CERK inhibitors might be a potential therapeutic tool in the treatment of allergic diseases.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alkenes / chemistry
  • Benzoquinones / chemistry
  • Benzoquinones / pharmacology*
  • Calcium / metabolism
  • Cell Degranulation / drug effects
  • Cell Membrane Permeability
  • Cells, Cultured
  • Chemistry, Organic / methods
  • Drug Evaluation, Preclinical / methods
  • Enzyme Inhibitors / chemical synthesis
  • Enzyme Inhibitors / pharmacology*
  • Humans
  • Immunoglobulin E / pharmacology
  • Isomerism
  • Mast Cells / drug effects*
  • Mast Cells / physiology
  • Phosphorylation / drug effects
  • Phosphotransferases (Alcohol Group Acceptor) / antagonists & inhibitors*
  • Phosphotransferases (Alcohol Group Acceptor) / metabolism
  • Toxicity Tests
  • Tyrosine / metabolism

Substances

  • Alkenes
  • Benzoquinones
  • Enzyme Inhibitors
  • F 12509A
  • Immunoglobulin E
  • Tyrosine
  • Phosphotransferases (Alcohol Group Acceptor)
  • ceramide kinase
  • Calcium