Nuclear Overhauser effect (NOE) enhancement of 11B NMR spectra of borane adducts in the solid state

J Am Chem Soc. 2006 May 31;128(21):6782-3. doi: 10.1021/ja0610939.

Abstract

A strong 11B {1H} nuclear Overhauser effect (NOE) enhancement can be observed in solid-state 11B NMR spectra of borane adducts, yielding fractional enhancements, fI{S} = (I - I0)/I0, of the magic angle spinning (MAS) NMR signal of up to 155%. This is an interesting and unusual observation as 11B (spin I = 3/2) is a quadrupolar nucleus and the corresponding NOE is completely absent in solution. More generally, it shows that the NOE may have a wider role to play in solid-state NMR studies of dynamics than has been envisaged hitherto.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Boranes / chemistry*
  • Boron / chemistry*
  • Magnetic Resonance Spectroscopy / methods*
  • Models, Chemical

Substances

  • Boranes
  • Boron