Reactions of alkyl-radicals with gold and silver nanoparticles in aqueous solutions

Phys Chem Chem Phys. 2006 Aug 14;8(30):3552-6. doi: 10.1039/b604140j. Epub 2006 Jun 20.

Abstract

Silver and gold nanoparticles are very efficient catalysts for the dimerization of methyl-radicals in aqueous solutions. The rate constants for the reaction of methyl-radicals with the gold and silver nanoparticles were measured and found to be 3.7 x 10(8) M(-1) s(-1) and 1.4 x 10(9) M(-1) s(-1), respectively. The results thus suggest that alkyl-radicals, also not reducing ones, are scavenged by these nanoparticles. This might explain the role, if such a role exists, of these nanoparticles in medical applications.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alkanes / chemistry*
  • Free Radicals / chemistry*
  • Gold / chemistry*
  • Nanostructures / chemistry*
  • Silver / chemistry*
  • Solutions
  • Water / chemistry*

Substances

  • Alkanes
  • Free Radicals
  • Solutions
  • Water
  • Silver
  • Gold