Performance of a fuel cell optimized for in situX-ray absorption experiments

J Synchrotron Radiat. 2007 May;14(Pt 3):276-81. doi: 10.1107/S0909049507013593. Epub 2007 Apr 11.

Abstract

A commercial fuel cell has been successfully modified to carry out X-ray absorption spectroscopy (XAS) measurements under optimized in operando conditions. The design is conceived for the performance of XAS experiments in transmission mode over a wide range of X-ray energies above 6 keV, owing to the reduced absorption of the cell. The wide angular aperture allows the collection of XAS in fluorescence mode and of X-ray diffraction patterns when needed. Details of the design of the cell and its performances are given. The quality of the extended X-ray absorption fine-structure spectra under working conditions has been verified at the ESRF and ELETTRA synchrotron radiation facilities, showing that relatively fast and low-noise transmission measurements on electrodes over a wide range of catalyst concentrations and energies are feasible.

MeSH terms

  • Electric Power Supplies*
  • Electrochemistry / instrumentation
  • Spectrometry, X-Ray Emission / instrumentation*
  • Synchrotrons