Polymeric micelles with glycolipid-like structure and multiple hydrophobic domains for mediating molecular target delivery of paclitaxel

Biomacromolecules. 2007 Aug;8(8):2450-6. doi: 10.1021/bm070365c. Epub 2007 Jul 28.

Abstract

Herein, polymeric micelles with glycolipid-like structure and about 40 nm diameter are prepared by self-aggregation from stearate-grafted chitosan oligosaccharides in aqueous medium. The micelles, with high degree of substitution (DS), present specific spatial structure with multiple hydrophobic "minor cores", and thus obtain excellent internalization into cancer cells and accumulation in cytoplasm. Furthermore, the micelles showed pH-sensitive properties, thus favoring intracellular delivery of encapsulated drug via endocytosis. The cell cytotoxicity of paclitaxel encapsulated in micelles was improved sharply and contributed to the increased intracellular delivery of the drug. The present micelles are a promising carrier candidate for targeting therapy of antitumor drugs with a cytoplasmic molecule target.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antineoplastic Agents, Phytogenic / administration & dosage*
  • Antineoplastic Agents, Phytogenic / chemistry
  • Antineoplastic Agents, Phytogenic / metabolism
  • Chitosan / chemistry*
  • Drug Carriers / chemistry*
  • Drug Carriers / metabolism
  • Endocytosis
  • Glycolipids / chemistry*
  • Glycolipids / metabolism
  • HeLa Cells
  • Humans
  • Hydrophobic and Hydrophilic Interactions
  • Micelles
  • Molecular Structure
  • Paclitaxel / administration & dosage*
  • Paclitaxel / chemistry
  • Paclitaxel / metabolism
  • Particle Size
  • Polymers / chemistry*
  • Polymers / metabolism
  • Water / chemistry

Substances

  • Antineoplastic Agents, Phytogenic
  • Drug Carriers
  • Glycolipids
  • Micelles
  • Polymers
  • Water
  • Chitosan
  • Paclitaxel