Identification of a second lipopolysaccharide in Porphyromonas gingivalis W50

J Bacteriol. 2008 Apr;190(8):2920-32. doi: 10.1128/JB.01868-07. Epub 2008 Feb 8.

Abstract

We previously described a cell surface anionic polysaccharide (APS) in Porphyromonas gingivalis that is required for cell integrity and serum resistance. APS is a phosphorylated branched mannan that shares a common epitope with posttranslational additions to some of the Arg-gingipains. This study aimed to determine the mechanism of anchoring of APS to the surface of P. gingivalis. APS was purified on concanavalin A affinity columns to minimize the loss of the anchoring system that occurred during chemical extraction. (1)H nuclear magnetic resonance spectroscopy of the lectin-purified APS confirmed the previous structure but also revealed additional signals that suggested the presence of a lipid A. This was confirmed by fatty acid analysis of the APS and matrix-assisted laser desorption ionization-time of flight mass spectrometry of the lipid A released by treatment with sodium acetate buffer (pH 4.5). Hence, P. gingivalis synthesizes two distinct lipopolysaccharide (LPS) macromolecules containing different glycan repeating units: O-LPS (with O-antigen tetrasaccharide repeating units) and A-LPS (with APS repeating units). Nonphosphorylated penta-acylated and nonphosphorylated tetra-acylated species were detected in lipid A from P. gingivalis total LPS and in lipid A from A-LPS. These lipid A species were unique to lipid A derived from A-LPS. Biological assays demonstrated a reduced proinflammatory activity of A-LPS compared to that of total LPS. Inactivation of a putative O-antigen ligase (waaL) at PG1051, which is required for the final step of LPS biosynthesis, abolished the linkage of both the O antigen and APS to the lipid A core of O-LPS and A-LPS, respectively, suggesting that WaaL in P. gingivalis has dual specificity for both O-antigen and APS repeating units.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Carbohydrates / analysis
  • Carbon-Oxygen Ligases / genetics
  • Carbon-Oxygen Ligases / metabolism*
  • Cell Line
  • Chromatography, Affinity
  • Gas Chromatography-Mass Spectrometry
  • Gene Deletion
  • Hemolysis
  • Humans
  • Lipid A / chemistry
  • Lipid A / isolation & purification
  • Lipids / analysis
  • Lipopolysaccharides / chemistry*
  • Lipopolysaccharides / isolation & purification*
  • Lipopolysaccharides / metabolism
  • Lipopolysaccharides / toxicity
  • Magnetic Resonance Spectroscopy
  • Microscopy, Electron, Transmission
  • O Antigens / chemistry
  • Porphyromonas gingivalis / chemistry*
  • Porphyromonas gingivalis / metabolism
  • Porphyromonas gingivalis / pathogenicity
  • Porphyromonas gingivalis / ultrastructure
  • Spectrometry, Mass, Matrix-Assisted Laser Desorption-Ionization

Substances

  • Carbohydrates
  • Lipid A
  • Lipids
  • Lipopolysaccharides
  • O Antigens
  • Carbon-Oxygen Ligases