Benzyl ether-linked glucuronide derivative of 10-hydroxycamptothecin designed for selective camptothecin-based anticancer therapy

J Med Chem. 2008 Mar 27;51(6):1740-6. doi: 10.1021/jm701151c. Epub 2008 Mar 5.

Abstract

A beta-glucuronidase-activated prodrug approach was applied to 10-hydroxycamptothecin, a Camptotheca alkaloid with promising antitumor activity but poor water solubility. We synthesized a glucuronide prodrug of 10-hydroxycamptothecin ( 7) in which glucuronic acid is connected via a self-immolative 3-nitrobenzyl ether linker to the 10-OH group of 10-hydroxycamptothecin. Compound 7 was 80 times more soluble than 10-hydroxycamptothecin in aqueous solution at pH 4.0 and was stable in human plasma. Prodrug 7 was 10- to 15-fold less toxic than the parent drug to four human tumor cell lines. In the presence of beta-glucuronidase, prodrug 7 could be activated to elicit similar cytotoxicity to the parent drug in tumor cells. Enzyme kinetic studies showed that Escherichia coli beta-glucuronidase had a quite low K m of 0.18 microM for compound 7 and exhibited 520 times higher catalytic efficiency for 7 than for 6 (a glucuronide prodrug of 9-aminocamptothecin). Molecular modeling studies predicted that compound 7 would have a higher binding affinity to human beta-glucuronidase than compound 6. Prodrug 7 may be useful for selective cancer chemotherapy by a prodrug monotherapy (PMT) or antibody-directed enzyme prodrug therapy (ADEPT) strategy.

MeSH terms

  • Antibodies, Neoplasm / chemistry
  • Antibodies, Neoplasm / pharmacology
  • Antibodies, Neoplasm / therapeutic use
  • Antineoplastic Agents / chemistry
  • Antineoplastic Agents / pharmacology
  • Antineoplastic Agents / therapeutic use
  • Binding, Competitive
  • Camptothecin / analogs & derivatives*
  • Camptothecin / chemistry
  • Camptothecin / pharmacology
  • Camptothecin / therapeutic use
  • Catalysis
  • Cell Line, Tumor
  • Cell Proliferation / drug effects
  • Drug Design
  • Drug Screening Assays, Antitumor
  • Escherichia coli / enzymology
  • Glucuronidase / chemistry
  • Glucuronidase / drug effects
  • Glucuronides / chemistry*
  • Humans
  • Kinetics
  • Models, Molecular
  • Molecular Structure
  • Neoplasms / drug therapy*
  • Phenyl Ethers / chemistry*
  • Prodrugs / chemistry
  • Prodrugs / pharmacology*
  • Prodrugs / therapeutic use*
  • Structure-Activity Relationship

Substances

  • Antibodies, Neoplasm
  • Antineoplastic Agents
  • Glucuronides
  • Phenyl Ethers
  • Prodrugs
  • 10-hydroxycamptothecin
  • Glucuronidase
  • Camptothecin