Alternative method for site-directed mutagenesis of complex polyketide synthase in Streptomyces albus JA3453

Acta Biochim Biophys Sin (Shanghai). 2008 Apr;40(4):319-26. doi: 10.1111/j.1745-7270.2008.00408.x.

Abstract

Sequence analysis of oxazolomycin (OZM) biosynthetic gene cluster from Streptomyces albus JA3453 revealed a gene, ozmH, encoding a hybrid polyketide and non-ribosomal peptide enzyme. Tandem ketosynthase (KS) domains (KS 10-1 and KS 10-2) were characterized and they show significant homology with known KSs. Using an alternative method that involves RecA-mediated homologous recombination, the negative selection marker sacB gene, and temperature-sensitive replications, site-directed mutagenesis of the catalytic triad amino acid cysteines were carried out in each of the tandem KS domains to test the function they play in OZM biosynthesis. HPLC-mass spectrometry analysis of the resulting mutant strains showed that KS 10-2 is essential for OZM biosynthesis but KS 10-1 is not indispensable and might serve as a "redundant" domain. These results confirmed the existence of an "extra domain" in complex polyketide synthase.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Enzyme Activation
  • Enzyme Stability
  • Mutagenesis, Site-Directed / methods*
  • Polyketide Synthases / chemistry*
  • Polyketide Synthases / genetics*
  • Polyketide Synthases / metabolism
  • Protein Engineering / methods*
  • Streptomyces / classification
  • Streptomyces / enzymology*
  • Streptomyces / genetics*
  • Structure-Activity Relationship

Substances

  • Polyketide Synthases