Production of biologically active forms of recombinant hepcidin, the iron-regulatory hormone

FEBS J. 2008 Aug;275(15):3793-803. doi: 10.1111/j.1742-4658.2008.06525.x. Epub 2008 Jun 28.

Abstract

Hepcidin is a liver produced cysteine-rich peptide hormone that acts as the central regulator of body iron metabolism. Hepcidin is synthesized under the form of a precursor, prohepcidin, which is processed to produce the biologically active mature 25 amino acid peptide. This peptide is secreted and acts by controlling the concentration of the membrane iron exporter ferroportin on intestinal enterocytes and macrophages. Hepcidin binds to ferroportin, inducing its internalization and degradation, thus regulating the export of iron from cells to plasma. The aim of the present study was to develop a novel method to produce human and mouse recombinant hepcidins, and to compare their biological activity towards their natural receptor ferroportin. Hepcidins were expressed in Escherichia coli as thioredoxin fusion proteins. The corresponding peptides, purified after cleavage from thioredoxin, were properly folded and contained the expected four-disulfide bridges without the need of any renaturation or oxidation steps. Human and mouse hepcidins were found to be biologically active, promoting ferroportin degradation in macrophages. Importantly, biologically inactive aggregated forms of hepcidin were observed depending on purification and storage conditions, but such forms were unrelated to disulfide bridge formation.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antimicrobial Cationic Peptides / biosynthesis*
  • Antimicrobial Cationic Peptides / isolation & purification
  • Antimicrobial Cationic Peptides / physiology
  • Base Sequence
  • Chromatography, High Pressure Liquid
  • DNA Primers
  • Electrophoresis, Polyacrylamide Gel
  • Hepcidins
  • Humans
  • Iron-Regulatory Proteins / biosynthesis*
  • Iron-Regulatory Proteins / isolation & purification
  • Iron-Regulatory Proteins / physiology
  • Mass Spectrometry / methods
  • Mice
  • Recombinant Proteins / biosynthesis
  • Recombinant Proteins / isolation & purification
  • Recombinant Proteins / metabolism

Substances

  • Antimicrobial Cationic Peptides
  • DNA Primers
  • HAMP protein, human
  • Hamp protein, mouse
  • Hepcidins
  • Iron-Regulatory Proteins
  • Recombinant Proteins