A Caco-2 cell based screening method for compounds interacting with MRP2 efflux protein

Eur J Pharm Biopharm. 2009 Feb;71(2):332-8. doi: 10.1016/j.ejpb.2008.08.010. Epub 2008 Aug 19.

Abstract

The aim of this work was to develop a screening method for MRP2 efflux substrates using the well-characterized, human-based intestinal Caco-2 cell model as a platform. MRP2 has a significant role in drug absorption and disposition and is known to co-operate with phase II metabolic enzymes. Caco-2 cells grown in a 96-well plate were loaded with non-fluorescent CDCFDA (diacetate ester of 5(6)-carboxy-2',7'-dichlorofluorescein), which is hydrolyzed to fluorescent CDCF by intracellular esterases. De-esterification in Caco-2 was comparable to that in porcine liver esterases. CDCFDA enters the cells passively, while CDCF is effluxed out of the cells by the apically localized MRP2 and/or basolateral MRPs. The method was optimized with regard to several factors. In the concluding protocol, Caco-2 cells are grown on clear 96-well plates for 8 days. The loading conditions were optimized to 10 min incubation with 5 microM CDCFDA. The highest responses were obtained for samples taken at t=30 min. The samples were analyzed in black 96-well plates with a fluorescence plate reader. The Caco-2 based method utilizing the probe pair CDCFDA/CDCF provides a fast screening tool for MRP2 substrates and/or inhibitors, along with compounds having metabolites formed in Caco-2 that interact with MRP2.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biological Transport
  • Caco-2 Cells
  • Fluoresceins / metabolism*
  • Fluorescent Dyes / metabolism
  • Humans
  • Models, Biological*
  • Multidrug Resistance-Associated Protein 2
  • Multidrug Resistance-Associated Proteins / drug effects
  • Multidrug Resistance-Associated Proteins / metabolism*
  • Pharmaceutical Preparations / metabolism

Substances

  • ABCC2 protein, human
  • Fluoresceins
  • Fluorescent Dyes
  • Multidrug Resistance-Associated Protein 2
  • Multidrug Resistance-Associated Proteins
  • Pharmaceutical Preparations
  • 5(6)-carboxy-2',7'-dichlorofluorescein