A diastereoselective route to 2,6-syn-disubstituted tetrahydropyrans: synthesis of the civet compound (+)-2-((2S,6S)-6-methyltetrahydro-2H-pyran-2-yl) acetic acid

Chem Commun (Camb). 2008 Nov 21:(43):5559-61. doi: 10.1039/b810231g. Epub 2008 Sep 30.

Abstract

A diastereoselective synthesis of 2,6-syn-disubstituted tetrahydropyrans has been developed based on the ability of furanyl-ether chiral centres to epimerise readily under acidic conditions. This novel methodology was applied to the synthesis of (+)-2-((2S,6S)-6-methyltetrahydro-2H-pyran-2-yl) acetic acid, a component of the African civet cat's glandular marking secretion.

MeSH terms

  • Acetates / chemical synthesis*
  • Acetates / chemistry
  • Molecular Conformation
  • Pyrans / chemical synthesis*
  • Pyrans / chemistry
  • Stereoisomerism

Substances

  • 2-((2S,6S)-6-methyltetrahydro-2H-pyran-2-yl) acetic acid
  • Acetates
  • Pyrans