Tubocapsanolide A inhibits transforming growth factor-beta-activating kinase 1 to suppress NF-kappaB-induced CCR7

J Biol Chem. 2009 Jan 30;284(5):2746-2754. doi: 10.1074/jbc.M806223200. Epub 2008 Dec 2.

Abstract

Withanolides are C(28) steroidal lactones isolated from plants that exhibit potent anti-cancer activity. The chemokine receptor CCR7 is important for lymphatic invasion of cancer cells and is overexpressed in metastatic breast cancer cells. A bioactive withanolide tubocapsanolide A (Tubo A) suppressed NF-kappaB-mediated CCR7 expression in breast cancer cells and attenuated their migration toward lymphatic endothelial cells. Chromatin immunoprecipitation assay confirmed that binding of NF-kappaBto the consensus site localized at the -398/-389 of human CCR7 promoter was repressed by Tubo A. Tubo A inhibited IkappaB kinase (IKK) and p38 kinase and downstream mitogen and stress-activated protein kinase 1 (MSK1) activity to reduce IkappaB degradation and to suppress NF-kappaB activation. Co-expression of IKK and MSK1 fully rescued Tubo A-induced inhibition. In addition, ectopic expression of transforming growth factor-beta-activating kinase (TAK1), the common upstream kinase of IKK and MSK1, also completely reversed the inhibition by Tubo A. Most importantly, Tubo A reduced NF-kappaB activation, CCR7 expression, and lymph node metastasis of breast cancer in vivo. We conclude that Tubo A inhibits TAK1 to repress NF-kappaB-induced CCR7 expression in breast cancer cells and suggest that Tubo A may be useful for the prevention of lymphatic invasion of breast cancer cells.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Base Sequence
  • Cell Line, Tumor
  • Chromatin Immunoprecipitation
  • DNA Primers
  • Ergosterol / analogs & derivatives*
  • Ergosterol / pharmacology
  • Flow Cytometry
  • Humans
  • MAP Kinase Kinase Kinases / antagonists & inhibitors*
  • NF-kappa B / antagonists & inhibitors*
  • NF-kappa B / genetics
  • NF-kappa B / physiology
  • Promoter Regions, Genetic
  • Receptors, CCR7 / antagonists & inhibitors*
  • Receptors, CCR7 / physiology
  • Reverse Transcriptase Polymerase Chain Reaction

Substances

  • CCR7 protein, human
  • DNA Primers
  • NF-kappa B
  • Receptors, CCR7
  • tubocapsanolide A
  • MAP Kinase Kinase Kinases
  • MAP kinase kinase kinase 7
  • Ergosterol