A catalytic asymmetric route to carbapenems

Org Lett. 2009 Aug 20;11(16):3606-9. doi: 10.1021/ol901269d.

Abstract

Efficient syntheses of N-acetyl thienamycin and epithienamycin A in their readily deprotected form are reported where three contiguous stereocenters are established in a single catalytic asymmetric azetidinone-forming reaction. These examples are a template for synthesizing C-5/C-6 cis or trans carbapenems with independent control of the C-8 stereocenter. A library of oxidatively and sterochemically defined azetidinone precursors to a variety of naturally occurring carbapenems and potential biosynthetic intermediates has been prepared to facilitate studies of carbapenem antibiotic biosynthesis.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Anti-Bacterial Agents / chemical synthesis*
  • Anti-Bacterial Agents / chemistry
  • Carbapenems / chemical synthesis*
  • Carbapenems / chemistry
  • Catalysis
  • Combinatorial Chemistry Techniques
  • Molecular Structure
  • Stereoisomerism

Substances

  • Anti-Bacterial Agents
  • Carbapenems