Sun light degradation of 4-chloroaniline in waters and its effect on toxicity. A high performance liquid chromatography - Diode array - Tandem mass spectrometry study

Environ Pollut. 2010 Feb;158(2):592-8. doi: 10.1016/j.envpol.2009.08.012. Epub 2009 Sep 20.

Abstract

This paper studies the degradation reactions that 4-chloroaniline can naturally undergo in waters for the action of sun light. 10.00 mg L(-1) 4-chloroaniline aqueous solution, without any addition of organic solvent, are undergone to photoirradiation under conditions that simulate sun light. The degradation pathway, followed by HPLC-DAD-MS/MS methods, is complex since the pollutant gives rise to many photoproducts: the predominant species are characterized by m/z values of 217 (P5) and 218 (P6) and are compatible with dimeric structures of 4-chloroaniline. Vibrio fischeri tests indicate that the photoproducts of 4-chloroaniline are characterized by a toxicity level significantly greater than the precursor.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Aliivibrio fischeri / drug effects
  • Aniline Compounds / chemistry*
  • Aniline Compounds / toxicity*
  • Chromatography, High Pressure Liquid / methods
  • Environmental Restoration and Remediation / methods*
  • Oxygen / analysis
  • Sunlight*
  • Tandem Mass Spectrometry / methods
  • Toxicity Tests
  • Water Pollutants, Chemical / chemistry*

Substances

  • Aniline Compounds
  • Water Pollutants, Chemical
  • Oxygen
  • 4-chloroaniline