Electrical sintering of silver nanoparticle ink studied by in-situ TEM probing

PLoS One. 2011 Feb 24;6(2):e17209. doi: 10.1371/journal.pone.0017209.

Abstract

Metallic nanoparticle inks are used for printed electronics, but to reach acceptable conductivity the structures need to be sintered, usually using a furnace. Recently, sintering by direct resistive heating has been demonstrated. For a microscopic understanding of this Joule heating sintering method, we studied the entire process in real time inside a transmission electron microscope equipped with a movable electrical probe. We found an onset of Joule heating induced sintering and coalescence of nanoparticles at power levels of 0.1-10 mW/μm³. In addition, a carbonization of the organic shells that stabilize the nanoparticles were found, with a conductivity of 4 10⁵ Sm⁻¹.

Publication types

  • Evaluation Study

MeSH terms

  • Air
  • Carbon / metabolism
  • Electron Probe Microanalysis / methods
  • Electroplating / methods*
  • Ink*
  • Materials Testing / methods
  • Metal Nanoparticles / chemistry*
  • Microscopy, Electron, Transmission / methods*
  • Models, Biological
  • Particle Size
  • Silver / chemistry*
  • Silver Compounds / chemical synthesis*
  • Silver Compounds / chemistry

Substances

  • Silver Compounds
  • Silver
  • Carbon