Passage from spin-polarized surface states to unpolarized quantum well states in topologically nontrivial Sb films

Phys Rev Lett. 2011 Jul 15;107(3):036802. doi: 10.1103/PhysRevLett.107.036802. Epub 2011 Jul 11.

Abstract

Topological materials have unusual surface spin properties including a net surface spin current protected by the bulk symmetry properties. When such materials are reduced to thin films, their gapless spin-polarized surface states must connect, by analytic continuation, to bulk-derived quantum-well states, which are spin-unpolarized in centrosymmetric systems. The nature of this passage in a model system, Sb films, is investigated. Angle-resolved photoemission shows a smooth transition, while calculations elucidate the correlated evolution of the spin and charge distributions in real space.