Trans, trans-muconic acid as a biomarker of occupational exposure to high-level benzene in China

J Occup Environ Med. 2011 Oct;53(10):1194-8. doi: 10.1097/JOM.0b013e31822cfd36.

Abstract

Objective: The work aimed to study the potential correlation between the high-level benzene exposure and its urinary metabolites S-phenylmercapturic acid (SPMA) and trans, trans-muconic acid (t,t-MA) in Chinese shoe-making workers.

Methods: Individual benzene-exposed levels were determined by gas chromatography analysis, urinary t,t-MA, and urinary SPMA were determined by high performance liquid chromatography-an ultraviolet detector and liquid chromatography/electrospray tandem mass spectrometry method, respectively.

Results: The concentration of benzene ranged from 2.57 to 146.11 mg/m³. And the correlation between benzene and t,t-MA was significantly higher than that of SPMA at the postshift, for example, the correlation coefficient was 0.905 and 0.537 for t,t-MA and SPMA, respectively. Moreover, The relative internal exposure index of t,t-MA (0.28 mg/g Cr: mg/m³) was more similar to the data supplied by American Conference of Governmental Industrial Hygienists compared to the index of SPMA (0.025 mg/g Cr:mg/m³).

Conclusions: t,t-MA appeared to be a more specific biomarker than SPMA at high-level benzene exposure.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetylcysteine / analogs & derivatives*
  • Acetylcysteine / urine
  • Adult
  • Air Pollutants, Occupational / analysis*
  • Benzene / analysis*
  • Benzene / metabolism
  • Biomarkers / urine
  • China
  • Female
  • Humans
  • Male
  • Occupational Exposure*
  • Sorbic Acid / analogs & derivatives*
  • Sorbic Acid / metabolism
  • Statistics, Nonparametric

Substances

  • Air Pollutants, Occupational
  • Biomarkers
  • muconic acid
  • S-phenyl-N-acetylcysteine
  • Benzene
  • Acetylcysteine
  • Sorbic Acid