Analysis of sexual assault evidence by desorption electrospray ionization mass spectrometry

J Mass Spectrom. 2013 Jul;48(7):774-8. doi: 10.1002/jms.3205.

Abstract

Desorption electrospray ionization mass spectrometry (DESI-MS) is employed in the forensic analysis of chemical components present in condoms and imaging of latent fingerprints as circumstantial evidence of sexual assault. Polymers such as nonoxynol-9, polyethylene glycol, and polydimethylsiloxane, as well as small molecules additives such as N-methylmorpholine, N-octylamine, N,N-dibutyl formamide, and isonox 132, commonly used in lubricated condom formulations, were successfully characterized by DESI. The results suggest that DESI-MS is useful for identification of this type of evidence, and it has advantages over conventional extractive techniques, in terms of speed of analysis and ease of use.

Keywords: DESI; ambient ionization; condoms; forensics; polymers.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amines / analysis
  • Amines / chemistry
  • Condoms*
  • Dermatoglyphics
  • Dimethylpolysiloxanes / analysis
  • Dimethylpolysiloxanes / chemistry
  • Forensic Medicine / methods*
  • Humans
  • Morpholines / analysis
  • Morpholines / chemistry
  • Nonoxynol / analysis
  • Nonoxynol / chemistry
  • Rubber / chemistry
  • Sex Offenses*
  • Spectrometry, Mass, Electrospray Ionization / methods*

Substances

  • Amines
  • Dimethylpolysiloxanes
  • Morpholines
  • 4-methylmorpholine
  • Nonoxynol
  • baysilon
  • Rubber
  • octylamine