Noninvasive molecular imaging of tuberculosis-associated inflammation with radioiodinated DPA-713

J Infect Dis. 2013 Dec 15;208(12):2067-74. doi: 10.1093/infdis/jit331. Epub 2013 Jul 30.

Abstract

Background: Increased expression of translocator protein (TSPO) is a feature of microglial and macrophage activation. Since activated macrophages are key components of tuberculosis-associated inflammation, we evaluated radioiodinated DPA-713, a synthetic ligand of TSPO, for in vivo imaging of host response.

Methods: Mice were infected with aerosolized Mycobacterium tuberculosis and evaluated using whole-body [(125)I]iodo-DPA-713 single-photon emission computed tomography (SPECT). Ex vivo biodistribution and correlative immunofluorescence studies were also performed.

Results: [(125)I]Iodo-DPA-713 SPECT imaging clearly delineated tuberculosis-associated pulmonary inflammation in live animals. Biodistribution studies confirmed radiotracer specificity for inflamed pulmonary tissues. Immunofluorescence studies demonstrated that TSPO is highly expressed in CD68(+) macrophages and phagocytic cells within tuberculosis lesions and that [(125)I]DPA-713 specifically accumulates within these cells. Coadministration of excess unlabelled DPA-713 abrogated both the SPECT and ex vivo fluorescence signals. Lesion-specific signal-to-noise ratios were significantly higher with [(125)I]iodo-DPA-713 SPECT (4.06 ± 0.52) versus [(18)F]fluorodeoxyglucose (FDG) positron emission tomography (PET) (2.00 ± 0.28) performed in the same mice (P = .004).

Conclusions: [(125)I]Iodo-DPA-713 accumulates specifically in tuberculosis-associated inflammatory lesions by selective retention within macrophages and phagocytic cells. [(125)I]Iodo-DPA-713 SPECT provides higher lesion-specific signal-to-noise ratios than [(18)F]FDG PET and may prove to be a more specific biomarker to monitor tuberculosis in situ.

Keywords: PET; macrophage; molecular imaging; pyrazolopyrimidine; translocator protein; tuberculosis.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Acetamides / chemistry*
  • Acetamides / pharmacokinetics
  • Animals
  • Female
  • Granuloma / pathology
  • Lung / pathology*
  • Macrophages / chemistry
  • Mice
  • Mice, Inbred BALB C
  • Mice, Inbred C3H
  • Molecular Imaging / methods*
  • Phagocytes / chemistry
  • Pneumonia / pathology
  • Pyrazoles / chemistry*
  • Pyrazoles / pharmacokinetics
  • Pyrimidines / chemistry*
  • Pyrimidines / pharmacokinetics
  • Receptors, GABA / metabolism
  • Tissue Distribution
  • Tomography, Emission-Computed, Single-Photon / methods*
  • Tuberculosis / pathology*

Substances

  • Acetamides
  • Bzrp protein, mouse
  • N,N-diethyl-2-(2-(4-methoxyphenyl)-5,7-dimethyl-pyrazolo(1,5-a)pyrimidin-3-yl)-acetamide
  • Pyrazoles
  • Pyrimidines
  • Receptors, GABA