Quantitative receptor-based imaging of tumor proliferation with the sigma-2 ligand [(18)F]ISO-1

PLoS One. 2013 Sep 20;8(9):e74188. doi: 10.1371/journal.pone.0074188. eCollection 2013.

Abstract

The sigma-2 receptor is expressed in higher density in proliferating (P) tumor cells versus quiescent (Q) tumor cells, thus providing an attractive target for imaging the proliferative status (i.e., P:Q ratio) of solid tumors. Here we evaluate the utility of the sigma-2 receptor ligand 2-(2-[(18)F]fluoroethoxy)-N-(4-(3,4-dihydro-6,7-dimethoxyisoquinolin-2(1H)-yl)butyl)-5-methyl-benzamide, [(18)F]ISO-1, in two different rodent models of breast cancer. In the first study, small animal Positron Emission Tomography (PET) imaging studies were conducted with [(18)F]ISO-1 and (18)FDG in xenografts of mouse mammary tumor 66 and tracer uptake was correlated with the in vivo P:Q ratio determined by flow cytometric measures of BrdU-labeled tumor cells. The second model utilized a chemically-induced (N-methyl-N-nitrosourea [MNU]) model of rat mammary carcinoma to correlate measures of [(18)F]ISO-1 and FDG uptake with MR-based volumetric measures of tumor growth. In addition, [(18)F]ISO-1 and FDG were used to assess the response of MNU-induced tumors to bexarotene and Vorozole therapy. In the mouse mammary 66 tumors, a strong linear correlation was observed between the [(18)F]ISO-1 tumor: background ratio and the proliferative status (P:Q ratio) of the tumor (R = 0.87). Similarly, measures of [(18)F]ISO-1 uptake in MNU-induced tumors significantly correlated (R = 0.68, P<0.003) with changes in tumor volume between consecutive MR imaging sessions. Our data suggest that PET studies of [(18)F]ISO-1 provide a measure of both the proliferative status and tumor growth rate, which would be valuable in designing an appropriate treatment strategy.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alkylating Agents / toxicity
  • Animals
  • Anticarcinogenic Agents / therapeutic use
  • Apoptosis / drug effects
  • Benzamides*
  • Bexarotene
  • Blotting, Western
  • Cell Proliferation / drug effects*
  • Female
  • Flow Cytometry
  • Fluorodeoxyglucose F18*
  • Humans
  • Image Processing, Computer-Assisted
  • Ligands*
  • Mammary Neoplasms, Animal / chemically induced
  • Mammary Neoplasms, Animal / diagnostic imaging*
  • Mammary Neoplasms, Animal / drug therapy
  • Mammary Neoplasms, Animal / metabolism
  • Methylnitrosourea / toxicity
  • Mice
  • Positron-Emission Tomography
  • Radiopharmaceuticals*
  • Rats
  • Receptors, sigma / metabolism*
  • Tetrahydronaphthalenes / therapeutic use
  • Triazoles / therapeutic use
  • Tumor Cells, Cultured

Substances

  • Alkylating Agents
  • Anticarcinogenic Agents
  • Benzamides
  • Ligands
  • Radiopharmaceuticals
  • Receptors, sigma
  • Tetrahydronaphthalenes
  • Triazoles
  • sigma-2 receptor
  • Fluorodeoxyglucose F18
  • vorozole
  • Methylnitrosourea
  • Bexarotene