Heating and microwave assisted SPPS of C-terminal acid peptides on trityl resin: the truth behind the yield

Amino Acids. 2013 Dec;45(6):1395-403. doi: 10.1007/s00726-013-1604-z. Epub 2013 Oct 19.

Abstract

Despite correct purity of crude peptides prepared on trityl resin by Fmoc/tBu microwave assisted solid phase peptide synthesis, surprisingly, lower yields than those expected were obtained while preparing C-terminal acid peptides. This could be explained by cyclization/cleavage through diketopiperazine formation during the second amino acid deprotection and third amino acid coupling. However, we provide here evidence that this is not the case and that this yield loss was due to high temperature promoted hydrolysis of the 2-chlorotrityl ester, yielding premature cleavage of the C-terminal acid peptides.

MeSH terms

  • Heating*
  • Microwaves*
  • Molecular Structure
  • Peptides / chemical synthesis*
  • Peptides / chemistry*
  • Peptides / isolation & purification
  • Resins, Synthetic / chemistry*

Substances

  • Peptides
  • Resins, Synthetic