Advances in the determination of nucleic acid conformational ensembles

Annu Rev Phys Chem. 2014:65:293-316. doi: 10.1146/annurev-physchem-040412-110059. Epub 2013 Dec 16.

Abstract

Conformational changes in nucleic acids play a key role in the way genetic information is stored, transferred, and processed in living cells. Here, we describe new approaches that employ a broad range of experimental data, including NMR-derived chemical shifts and residual dipolar couplings, small-angle X-ray scattering, and computational approaches such as molecular dynamics simulations to determine ensembles of DNA and RNA at atomic resolution. We review the complementary information that can be obtained from diverse sets of data and the various methods that have been developed to combine these data with computational methods to construct ensembles and assess their uncertainty. We conclude by surveying RNA and DNA ensembles determined using these methods, highlighting the unique physical and functional insights obtained so far.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Review

MeSH terms

  • Animals
  • DNA / chemistry*
  • Humans
  • Molecular Dynamics Simulation
  • Nuclear Magnetic Resonance, Biomolecular / methods*
  • Nucleic Acid Conformation
  • RNA / chemistry*
  • Scattering, Small Angle*
  • X-Ray Diffraction / methods*

Substances

  • RNA
  • DNA