Cationic cyclizations and rearrangements promoted by a heterogeneous gold catalyst

Org Lett. 2014 Feb 7;16(3):800-3. doi: 10.1021/ol403542k. Epub 2014 Jan 16.

Abstract

A heterogeneous gold catalyst with remarkable activity for promoting the electrophilic reactions of aryl vinyl ketones and aryl dienyl ketones is described. The catalyst is easy to prepare, is robust, and can be recycled. Low loadings are effective for different types of cationic reactions, including Nazarov cyclizations, lactonizations, and [1,2] shifts.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Catalysis
  • Cations / chemistry*
  • Cyclization
  • Gold / chemistry*
  • Ketones / chemistry*
  • Molecular Structure
  • Stereoisomerism

Substances

  • Cations
  • Ketones
  • Gold