Continuous throughput and long-term observation of single-molecule FRET without immobilization

Nat Methods. 2014 Mar;11(3):297-300. doi: 10.1038/nmeth.2809. Epub 2014 Jan 19.

Abstract

We present an automated microfluidic platform that performs multisecond observation of single molecules with millisecond time resolution while bypassing the need for immobilization procedures. With this system, we confine biomolecules to a thin excitation field by reversibly collapsing microchannels to nanochannels. We demonstrate the power of our method by studying a variety of complex nucleic acid and protein systems, including DNA Holliday junctions, nucleosomes and human transglutaminase 2.

Publication types

  • Evaluation Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Automation
  • Fluorescence Resonance Energy Transfer*
  • GTP-Binding Proteins / genetics
  • Humans
  • Microfluidics / instrumentation*
  • Microfluidics / methods*
  • Models, Molecular
  • Protein Glutamine gamma Glutamyltransferase 2
  • Transglutaminases / genetics

Substances

  • Protein Glutamine gamma Glutamyltransferase 2
  • Transglutaminases
  • GTP-Binding Proteins