Absolute and relative quantification of RNA modifications via biosynthetic isotopomers

Nucleic Acids Res. 2014 Oct;42(18):e142. doi: 10.1093/nar/gku733. Epub 2014 Aug 16.

Abstract

In the resurging field of RNA modifications, quantification is a bottleneck blocking many exciting avenues. With currently over 150 known nucleoside alterations, detection and quantification methods must encompass multiple modifications for a comprehensive profile. LC-MS/MS approaches offer a perspective for comprehensive parallel quantification of all the various modifications found in total RNA of a given organism. By feeding (13)C-glucose as sole carbon source, we have generated a stable isotope-labeled internal standard (SIL-IS) for bacterial RNA, which facilitates relative comparison of all modifications. While conventional SIL-IS approaches require the chemical synthesis of single modifications in weighable quantities, this SIL-IS consists of a nucleoside mixture covering all detectable RNA modifications of Escherichia coli, yet in small and initially unknown quantities. For absolute in addition to relative quantification, those quantities were determined by a combination of external calibration and sample spiking of the biosynthetic SIL-IS. For each nucleoside, we thus obtained a very robust relative response factor, which permits direct conversion of the MS signal to absolute amounts of substance. The application of the validated SIL-IS allowed highly precise quantification with standard deviations<2% during a 12-week period, and a linear dynamic range that was extended by two orders of magnitude.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Carbon Isotopes
  • Chromatography, Liquid* / standards
  • Escherichia coli / metabolism
  • Nucleosides / chemistry
  • Nucleosides / metabolism
  • Pseudouridine / analysis
  • RNA / chemistry*
  • Reference Standards
  • Tandem Mass Spectrometry* / standards

Substances

  • Carbon Isotopes
  • Nucleosides
  • Pseudouridine
  • RNA