Divergent total synthesis of triptolide, triptonide, tripdiolide, 16-hydroxytriptolide, and their analogues

J Org Chem. 2014 Nov 7;79(21):10110-22. doi: 10.1021/jo501744j. Epub 2014 Oct 24.

Abstract

A divergent route was developed for the formal total synthesis of triptolide, triptonide, and tripdiolide, as well as a total synthesis of 16-hydroxytriptolide and their analogues in an enantioselective form. Common advanced intermediate 5 was concisely assembled by employing an indium(III)-catalyzed cationic polycyclization reaction and a palladium-catalyzed carbonylation-lactone formation reaction as key steps. This advanced intermediate was readily converted to the above natural products by using palladium-catalyzed cross-coupling or the Claisen rearrangement reaction as key steps. Additionally, preliminary structure-cytotoxic activity relationship studies of C13 suggested that it might be a new modification site that could still retain the cytotoxicity.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Catalysis
  • Diterpenes / chemical synthesis*
  • Diterpenes / chemistry
  • Epoxy Compounds / chemical synthesis
  • Epoxy Compounds / chemistry
  • Indium / chemistry
  • Lactones / chemistry*
  • Palladium / chemistry
  • Phenanthrenes / chemical synthesis*
  • Phenanthrenes / chemistry
  • Triterpenes / chemical synthesis*
  • Triterpenes / chemistry

Substances

  • Diterpenes
  • Epoxy Compounds
  • Lactones
  • Phenanthrenes
  • Triterpenes
  • Indium
  • 16-hydroxytriptolide
  • triptolide
  • triptonide
  • Palladium
  • tripdiolide