β/δ-PrIT1, a highly insecticidal toxin from the venom of the Brazilian spider Phoneutria reidyi (F.O. Pickard-Cambridge, 1897)

Toxicon. 2015 Sep 15:104:73-82. doi: 10.1016/j.toxicon.2015.07.010. Epub 2015 Jul 26.

Abstract

A potent insecticidal toxin, β/δ-PrIT1, molecular mass of 5598.86 [M+H](+), was characterized from Phoneutria reidyi spider venom. Its partial amino acid sequence showed high similarity with insecticidal spider toxins from the genus Phoneutria. β/δ-PrIT1 was very toxic (LD50 = 4 nmol/g) to flies (Musca domestica), but not to mice (Mus musculus). Kinetic studies showed that (125)I-β/δ-PrIT1 binds to two distinct sites in insect sodium channels, with close affinity (Kd1 = 34.7 pM and Kd2 = 35.1 pM). Its association is rather fast (t1/2(1) = 1.4 min, t1/2(2) = 8.5 min) and its dissociation is a slower process (t1/2(1) = 5.4 min, t1/2(2) = 32.8 min). On rat brain synaptosomes β/δ-PrIT1 partially competed (∼30%) with the beta-toxin (125)I-CssIV, but did not compete with the alpha-toxin of reference (125)I-AaII, nor with the beta-toxin (125)I-TsVII. On cockroach nerve cord synaptosomes, β/δ-PrIT1 did not compete with the anti-insect toxin (125)I-LqqIT1, but it competed (IC50 = 80 pM) with the "alpha-like" toxin (125)I-BomIV. In cockroach neurons, β/δ-PrIT1 inhibited the inactivation of Nav-channels and it shifted the sodium channel activation to hyperpolarizing potentials. These results indicate two different binding sites for β/δ-PrIT1, leading to two different pharmacological responses. β/δ-PrIT1 is one of the most toxic spider toxins to insects without apparent toxicity to mammals, and provide new model for the development of insecticides.

Keywords: Anti-insect toxins; Phoneutria reidyi; Spider venoms; Voltage-gated sodium channels.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Binding Sites
  • Brazil
  • Cockroaches / cytology
  • Cockroaches / drug effects
  • Diptera / drug effects
  • Female
  • Insecticides / chemistry
  • Insecticides / pharmacology*
  • Male
  • Mice
  • Neurons / drug effects
  • Neurons / metabolism
  • Rats
  • Rats, Wistar
  • Sodium Channels / metabolism
  • Spider Venoms / chemistry
  • Spider Venoms / pharmacology*
  • Spiders / chemistry*
  • Synaptosomes / metabolism*

Substances

  • Insecticides
  • Sodium Channels
  • Spider Venoms