Development of GABAA Receptor Subtype-Selective Imidazobenzodiazepines as Novel Asthma Treatments

Mol Pharm. 2016 Jun 6;13(6):2026-38. doi: 10.1021/acs.molpharmaceut.6b00159. Epub 2016 May 10.

Abstract

Recent studies have demonstrated that subtype-selective GABAA receptor modulators are able to relax precontracted human airway smooth muscle ex vivo and reduce airway hyper-responsiveness in mice upon aerosol administration. Our goal in this study was to investigate systemic administration of subtype-selective GABAA receptor modulators to alleviate bronchoconstriction in a mouse model of asthma. Expression of GABAA receptor subunits was identified in mouse lungs, and the effects of α4-subunit-selective GABAAR modulators, XHE-III-74EE and its metabolite XHE-III-74A, were investigated in a murine model of asthma (ovalbumin sensitized and challenged BALB/c mice). We observed that chronic treatment with XHE-III-74EE significantly reduced airway hyper-responsiveness. In addition, acute treatment with XHE-III-74A but not XHE-III-74EE decreased airway eosinophilia. Immune suppressive activity was also shown in activated human T-cells with a reduction in IL-2 expression and intracellular calcium concentrations [Ca(2+)]i in the presence of GABA or XHE-III-74A, whereas XHE-III-74EE showed only partial reduction of [Ca(2+)]i and no inhibition of IL-2 secretion. However, both compounds significantly relaxed precontracted tracheal rings ex vivo. Overall, we conclude that the systemic delivery of a α4-subunit-selective GABAAR modulator shows good potential for a novel asthma therapy; however, the pharmacokinetic properties of this class of drug candidates have to be improved to enable better beneficial systemic pharmacodynamic effects.

Keywords: GABA; GABAA receptor; XHE-III-74A; XHE-III-74EE; airway smooth muscle; asthma; eosinophilia; inflammation.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, N.I.H., Extramural

MeSH terms

  • Animals
  • Asthma / drug therapy*
  • Asthma / metabolism
  • Benzodiazepines / pharmacology*
  • Cell Line, Tumor
  • Disease Models, Animal
  • Female
  • Guinea Pigs
  • Humans
  • Interleukin-2 / metabolism
  • Jurkat Cells
  • Male
  • Mice
  • Mice, Inbred BALB C
  • Muscle, Smooth / drug effects
  • Muscle, Smooth / metabolism
  • Ovalbumin / administration & dosage
  • Receptors, GABA-A / metabolism*
  • Respiratory System / drug effects
  • Respiratory System / metabolism
  • T-Lymphocytes / drug effects
  • T-Lymphocytes / metabolism
  • Xenopus laevis

Substances

  • Interleukin-2
  • Receptors, GABA-A
  • Benzodiazepines
  • Ovalbumin