Evaluation of toxicity and estrogenicity of the landfill-concentrated leachate during advanced oxidation treatment: chemical analyses and bioanalytical tools

Environ Sci Pollut Res Int. 2016 Aug;23(16):16015-24. doi: 10.1007/s11356-016-6669-2. Epub 2016 May 4.

Abstract

Landfill-concentrated leachate from membrane separation processes is a potential pollution source for the surroundings. In this study, the toxicity and estrogenicity potentials of concentrated leachate prior to and during UV-Fenton and Fenton treatments were assessed by a combination of chemical (di (2-ethylhexyl) phthalate and dibutyl phthalate were chosen as targets) and biological (Daphnia magna, Chlorella vulgaris, and E-screen assay) analyses. Removal efficiencies of measured di (2-ethylhexyl) phthalate and dibutyl phthalate were more than 97 % after treatment with the two methods. Biological tests showed acute toxicity effects on D. magna tests in untreated concentrated leachate samples, whereas acute toxicity on C. vulgaris tests was not observed. Both treatment methods were found to be efficient in reducing acute toxicity effects on D. magna tests. The E-screen test showed concentrated leachate had significant estrogenicity, UV-Fenton and Fenton treatment, especially the former, were effective methods for reducing estrogenicity of concentrated leachate. The EEQchem (estradiol equivalent concentration) of all samples could only explain 0.218-5.31 % range of the EEQbio. These results showed that UV-Fenton reagent could be considered as a suitable method for treatment of concentrated leachate, and the importance of the application of an integrated (biological + chemical) analytical approach for a comprehensive evaluation of treatment suitability.

Keywords: Acute toxicity; Advanced treatment; Chemical analysis; Estrogenicity; Landfill-concentrated leachate; MCF-7 cell line.

MeSH terms

  • Animals
  • Chlorella vulgaris / drug effects
  • Daphnia / drug effects
  • Dibutyl Phthalate* / chemistry
  • Dibutyl Phthalate* / radiation effects
  • Dibutyl Phthalate* / toxicity
  • Diethylhexyl Phthalate* / chemistry
  • Diethylhexyl Phthalate* / radiation effects
  • Diethylhexyl Phthalate* / toxicity
  • Estrogens* / chemistry
  • Estrogens* / radiation effects
  • Estrogens* / toxicity
  • Hydrogen Peroxide / chemistry*
  • Iron / chemistry*
  • Oxidation-Reduction
  • Ultraviolet Rays*
  • Waste Disposal Facilities
  • Waste Disposal, Fluid
  • Water Pollutants, Chemical* / chemistry
  • Water Pollutants, Chemical* / radiation effects
  • Water Pollutants, Chemical* / toxicity

Substances

  • Estrogens
  • Fenton's reagent
  • Water Pollutants, Chemical
  • Dibutyl Phthalate
  • Hydrogen Peroxide
  • Diethylhexyl Phthalate
  • Iron