The first catalytic asymmetric cycloadditions of imines with an enolisable anhydride

Org Biomol Chem. 2016 Aug 7;14(29):6955-9. doi: 10.1039/c6ob00048g. Epub 2016 Jul 6.

Abstract

The first catalytic, asymmetric reactions of imines with homophthalic anhydride to form disubstituted 3,4-dihydroisoquinolones are reported. The use of N-mesyl aldimines is key, as more basic imines undergo rapid uncatalysed reactions, while imines possessing larger N-sulphonyl substituents form lactams with lower ee.

MeSH terms

  • Anhydrides / chemistry*
  • Catalysis
  • Cycloaddition Reaction
  • Imines / chemistry*
  • Isoquinolines / chemical synthesis*
  • Isoquinolines / chemistry
  • Molecular Structure

Substances

  • Anhydrides
  • G 1616
  • Imines
  • Isoquinolines