A conserved amino acid residue critical for product and substrate specificity in plant triterpene synthases

Proc Natl Acad Sci U S A. 2016 Jul 26;113(30):E4407-14. doi: 10.1073/pnas.1605509113. Epub 2016 Jul 13.

Abstract

Triterpenes are structurally complex plant natural products with numerous medicinal applications. They are synthesized through an origami-like process that involves cyclization of the linear 30 carbon precursor 2,3-oxidosqualene into different triterpene scaffolds. Here, through a forward genetic screen in planta, we identify a conserved amino acid residue that determines product specificity in triterpene synthases from diverse plant species. Mutation of this residue results in a major change in triterpene cyclization, with production of tetracyclic rather than pentacyclic products. The mutated enzymes also use the more highly oxygenated substrate dioxidosqualene in preference to 2,3-oxidosqualene when expressed in yeast. Our discoveries provide new insights into triterpene cyclization, revealing hidden functional diversity within triterpene synthases. They further open up opportunities to engineer novel oxygenated triterpene scaffolds by manipulating the precursor supply.

Keywords: cyclization; mutants; natural products; plant defense; terpenes.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Amino Acids / chemistry
  • Amino Acids / genetics*
  • Avena / enzymology
  • Avena / genetics
  • Avena / metabolism
  • Conserved Sequence / genetics
  • Cyclization
  • Intramolecular Transferases / chemistry
  • Intramolecular Transferases / genetics*
  • Intramolecular Transferases / metabolism
  • Models, Molecular
  • Molecular Structure
  • Mutation
  • Plant Proteins / chemistry
  • Plant Proteins / genetics*
  • Plant Proteins / metabolism
  • Protein Domains
  • Sequence Homology, Amino Acid
  • Substrate Specificity
  • Triterpenes / chemistry
  • Triterpenes / metabolism*

Substances

  • Amino Acids
  • Plant Proteins
  • Triterpenes
  • Intramolecular Transferases
  • 2,3-oxidosqualene-beta-amyrin-cyclase