Elaboration of Sterically Hindered δ-Lactones through Ring-Closing Metathesis: Application to the Synthesis of the C1-C27 Fragment of Hemicalide

J Org Chem. 2016 Dec 16;81(24):12275-12290. doi: 10.1021/acs.joc.6b02208. Epub 2016 Dec 5.

Abstract

The synthesis of the C1-C27 fragment of hemicalide, a marine metabolite displaying a unique potent antiproliferative activity, has been accomplished. The synthetic approach highlights a remarkably efficient ring-closing metathesis reaction catalyzed by Nolan ruthenium indenylidene complexes to elaborate the highly substituted δ-lactone framework.

Publication types

  • Research Support, Non-U.S. Gov't